Publications

Research Publications

Selected peer-reviewed publications from my research. Connect with me on academic platforms:

Publication Type

Research Area

Physics-informed machine learning exploration of Na storage mechanisms in disordered carbon

Rampal, Nikhil, Weitzner, Stephen E, Omenya, Fredrick, Wood, Marissa, Reed, David M, Li, Xiaolin, Lee, Jonathan RI, Wan, Liwen F

Energy Storage Materials, 104967, 2026

Using machine learning to uncover sodium storage mechanisms in carbon-based materials for next-generation batteries.

Energy Storage Machine Learning

Mechanistic Insights into Defect-Mediated Crystallization Revealed by Lattice Strain Evolution

Yuan, Ke, Weber, Juliane, Rampal, Nikhil, Fang, Zhengwu, You, Jiahui, Boebinger, Matthew G, Zhang, Rui, Cha, Wonsuk, Anovitz, Lawrence M, Lee, Sang Soo, et al.

Journal of the American Chemical Society, 2026

Investigation of defect-mediated crystallization processes through the lens of lattice strain evolution.

Geochemical Systems

Nuclear quantum effects of metal surface-mediated C--H activation

Bunting, Rhys J, Shepherd, Sam, Rampal, Nikhil, Akhade, Sneha, Wilkins, David M, Pham, Tuan Anh

Physical Chemistry Chemical Physics, 27(30), 16051-16056, 2025

Exploring quantum effects in carbon-hydrogen bond activation on metal surfaces.

Extreme Conditions

Cross-Scale Modeling and Experimental Integration for Advancing Cathode Electrolyte Interphase Studies

Weitzner, Stephen E, Wang, Bo, Rampal, Nikhil, Jeong, Wonseok, Yuan, Suyue, Zhang, Shenli, Bucci, Giovanna, Adelstein, Nicole, Yan, Shan, Marschilok, Amy C, et al.

Energy Storage Materials, 104368, 2025

Multiscale approach to understanding cathode-electrolyte interfaces in lithium-ion batteries.

Energy Storage

Microstructure-Dependent Sodium Storage Mechanisms in Hard Carbon Anodes

Kitsu Iglesias, Luis, Marks, Samuel D, Rampal, Nikhil, Antonio, Emma N, de Ferreira de Menezes, Rafael, Zhang, Liang, Olds, Daniel, Weitzner, Stephen E, Sprenger, Kayla G, Wan, Liwen F, et al.

Small, 2505561, 2025

Investigation of how microstructure affects sodium storage in hard carbon battery anodes.

Energy Storage

How are Heterogeneous Nucleation Rate Observations Influenced by Instrument Resolution?

You, Jiahui, Yuan, Ke, Rampal, Nikhil, Stack, Andrew G, Starchenko, Vitalii

ACS Applied Materials & Interfaces, 17(11), 17492-17500, 2025

Analysis of how experimental instrument resolution affects observed nucleation rates.

Geochemical Systems

Iron Impurity Impairs the CO2 Capture Performance of MgO

Yuan, Ke, Rampal, Nikhil, Adapa, Sai, Evans, Barbara R, Bracco, Jacquelyn N, Boebinger, Matthew G, Stack, Andrew G, Weber, Juliane

ACS Applied Materials & Interfaces, 16(46), 64233-64243, 2024

Using microscopy and machine learning to understand how iron impurities affect carbon capture materials.

Geochemical Systems Machine Learning

Structural and transport properties of battery electrolytes at sub-zero temperatures

Rampal, Nikhil, Weitzner, Stephen E, Cho, Seongkoo, Orme, Christine A, Worsley, Marcus A, Wan, Liwen F

Energy & Environmental Science, 2024

Investigation of how battery electrolytes perform at extremely low temperatures, revealing critical structural and transport properties.

Energy Storage

Ion Correlations Decrease Particle Aggregation Rate by Increasing Hydration Forces at Interfaces

Butreddy, Pravalika, Heo, Jaeyoung, Rampal, Nikhil, Liu, Tingting, Liu, Lili, Smith, William, Zhang, Xin, Prange, Micah P, Legg, Benjamin A, Schenter, Gregory K, De Yoreo, James J, Chun, Jaehun, Stack, Andrew G, Nakouzi, Elias

ACS nano, 2024

Study of how ion correlations influence particle aggregation through hydration force effects.

Geochemical Systems

Impact of magnetic and electric fields on the free energy to form a calcium carbonate ion-pair

Yuan, Ke, Rampal, Nikhil, Du, Xuewei, Shu, Fangjun, Wang, Yanxing, Wang, Huiyao, Stack, Andrew G, Ishai, Paul Ben, Anovitz, Lawrence M, Xu, Pei

Physical Chemistry Chemical Physics, 2024

Investigation of how electromagnetic fields affect calcium carbonate formation energetics.

Geochemical Systems

Variations in proton transfer pathways and energetics on pristine and defect-rich quartz surfaces in water

Yuan, Ke, Rampal, Nikhil, Irle, Stephan, Criscenti, Louise J, Lee, Sang Soo, Adapa, Sai, Stack, Andrew G

Journal of Colloid and Interface Science, 666, 232-243, 2024

Study of proton transfer mechanisms at quartz surfaces with varying defect concentrations.

Geochemical Systems

Molecular Mechanisms of Sorbed Ion Effects during Boehmite Particle Aggregation

Liu, Tingting, Rampal, Nikhil, Nakouzi, Elias, Legg, Benjamin A, Chun, Jaehun, Liu, Lili, Schenter, Gregory K, De Yoreo, James J, Anovitz, Lawrence M, Stack, Andrew G

Langmuir, 40(17), 8791-8805, 2024

Investigation of how sorbed ions influence particle aggregation at the molecular level.

Geochemical Systems

Testing the hypothesis that solvent exchange limits the rates of calcite growth and dissolution

Rampal, Nikhil, Wang, Hsiu-Wen, Brady, Alexander B, Borreguero, Jose M, Biriukov, Denys, Mamontov, Eugene, Stack, Andrew G

RSC advances, 14(22), 15743-15754, 2024

Comprehensive testing of the solvent exchange limitation hypothesis in mineral growth and dissolution.

Geochemical Systems

Assessing an aqueous flow cell designed for in situ crystal growth under X-ray nanotomography and effects of radiolysis products

Yuan, Ke, Starchenko, Vitalii, Rampal, Nikhil, Yang, Fengchang, Xiao, Xianghui, Stack, Andrew G

Journal of Synchrotron Radiation, 30(3), 634-642, 2023

Design and assessment of a flow cell for studying crystal growth with X-ray imaging.

Geochemical Systems

The evolution of solvation symmetry and composition in Zn halide aqueous solutions from dilute to extreme concentrations

Dhakal, Diwash, Driscoll, Darren M, Govind, Niranjan, Stack, Andrew G, Rampal, Nikhil, Schenter, Gregory, Mundy, Christopher J, Fister, Timothy T, Fulton, John L, Balasubramanian, Mahalingam, et al.

Physical Chemistry Chemical Physics, 25(34), 22650-22661, 2023

Study of solvation structures in zinc halide solutions across concentration ranges.

Geochemical Systems

Exploring Reactivity in Aqueous Solutions and at Mineral-Water Interfaces Through the Lens of Rare Event Theory

Rampal, Nikhil

PhD Thesis, Columbia University, 2023

Doctoral thesis on using rare event theory to understand geochemical processes.

Geochemical Systems

In situ observations of barium sulfate nucleation in nanopores

Brady, Alexander B, Weber, Juliane, Yuan, Ke, Allard, Lawrence F, Avina, Omar, Ogaz, Ramon, Chang, Yao-Jen, Rampal, Nikhil, Starchenko, Vitalii, Rother, Gernot, et al.

Crystal Growth & Design, 22(12), 6941-6951, 2022

Direct observation of nucleation processes confined within nanoporous environments.

Geochemical Systems

Synergistic Enhancement of Lead and Selenate Uptake at the Barite (001)--Water Interface

Yang, Peng, Rampal, Nikhil, Weber, Juliane, Bracco, Jacquelyn N, Fenter, Paul, Stack, Andrew G, Lee, Sang Soo

Environmental Science & Technology, 56(23), 16801-16810, 2022

Study of how barite surfaces interact with and remove multiple contaminants simultaneously.

Geochemical Systems

The "good," the "bad," and the "hidden" in neutron scattering and molecular dynamics of ionic aqueous solutions

Biriukov, Denys, Wang, Hsiu-Wen, Rampal, Nikhil, Tempra, Carmelo, Kula, Patrik, Neuefeind, Joerg C, Stack, Andrew G, Předota, Milan

The Journal of Chemical Physics, 156(19), 2022

Critical analysis of neutron scattering techniques and MD simulations for ionic solutions.

Geochemical Systems

Frustrated Coulombic and cation size effects on nanoscale boehmite aggregation

Anovitz, Lawrence M, Huestis, P, Rampal, Nikhil, Stack, Andrew G, LaVerne, JA, Zhang, X, Schenter, GK, Chun, J, Legg, BA, Liu, L, et al.

The Journal of Physical Chemistry C, 126(9), 4391-4414, 2022

Investigation of electrostatic and size effects in mineral particle aggregation.

Geochemical Systems

Solution and interface structure and dynamics in geochemistry: Gateway to link elementary processes to mineral nucleation and growth

Wang, Hsiu-Wen, Yuan, Ke, Rampal, Nikhil, Stack, Andrew G

Crystal Growth & Design, 22(1), 853-870, 2021

Review linking molecular-scale processes to macroscopic mineral formation.

Geochemical Systems

Local molecular environment drives speciation and reactivity of ion complexes in concentrated salt solution

Rampal, Nikhil, Wang, Hsiu-Wen, Biriukov, Denys, Brady, Alexander B, Neuefeind, Joerg C, Předota, Milan, Stack, Andrew G

Journal of Molecular Liquids, 340, 116898, 2021

Study of how local environment affects ion behavior in concentrated solutions.

Geochemical Systems

Density functional tight-binding simulations reveal the presence of surface defects on the quartz (101)--water interface

Yuan, Ke, Rampal, Nikhil, Fenter, Paul, Kubicki, James D, Stack, Andrew G, Irle, Stephan

The Journal of Physical Chemistry C, 125(29), 16246-16255, 2021

Computational study revealing defect structures at mineral-water interfaces.

Geochemical Systems

Opposing effects of impurity ion Sr2+ on the heterogeneous nucleation and growth of barite (BaSO4)

Yuan, Ke, Starchenko, Vitalii, Rampal, Nikhil, Yang, Fengchang, Yang, Xiaogang, Xiao, Xianghui, Lee, Wah-Keat, Stack, Andrew G

Crystal Growth & Design, 21(10), 5828-5839, 2021

Study of how impurity ions can have contradictory effects on mineral formation processes.

Geochemical Systems

Integrated Machine Learning-Molecular Dynamics Framework for Electrolyte Property Prediction

Sagireddy, Srikant, Rampal, Nikhil, Weitzner, Stephen E, Wan, Liwen F

Under Review

Framework combining machine learning and molecular dynamics to predict electrolyte properties.

Energy Storage Machine Learning

Elucidating Li transport mechanism in disordered LiF from machine-learning molecular dynamic simulations

Yuan, Suyue, Rampal, Nikhil, Adelstein, Nicole, Wan, Liwen F

Under Internal Review

Investigation of lithium transport in disordered structures using ML-based simulations.

Energy Storage Machine Learning

Nanoscale Structural and Transport Fluctuations in the Electric Double Layer: Critical Drivers of Vanadium Redox Flow Battery Performance

Rampal, Nikhil, Weitzner, Stephen E, Sun, Wenyu, Hollas, Aaron, Murugesan, Vijayakumar, Reed, David M, van Buuren, Tony, Lee, Jonathon R I, Wan, Liwen F

Under Internal Review

Study of electric double layer properties affecting flow battery performance.

Energy Storage

Resolving Competing Effects in Battery Systems via Atomistic Simulations

Rampal, Nikhil, Weitzner, Stephen E, Cho, Seongkoo, Orme, Christine A, Worsley, Marcus A, Wan, Liwen F

Under Internal Review

Using computational methods to untangle complex competing effects in battery materials.

Energy Storage

High pressure phase stability and melt in shock-compressed titanium

Singh, Saransh, Paul, Reetam, Rampal, Nikhil, Bunting, Rhys J, Hamel, Sebastien, Pulver, Nathan, McGuire, Chistopher P, Clarke, Samantha M, Coleman, Amy, Vennari, Cara, et al.

Under Internal Review

Investigation of titanium behavior under extreme pressure and shock compression.

Extreme Conditions

Saturation Dependent Nucleation Pathways and Phase Transitions

Rampal, Nikhil, Wang, Hsiu-Wen, Yuan Ke, Karmakar, Tarak, Parinello, Michelle, Stack, Andrew G.

In preparation

Study of how saturation levels affect mineral formation pathways.

Geochemical Systems

Beyond Classical Nucleation Theory: Molecular Insights into Non-Classical Pathways of Sparingly Soluble Salts

Rampal, Nikhil, Wang, Hsiu-Wen, Yuan, Ke, Stack, Andrew

American Conference of Crystal Growth and Epitaxy, 2025

Session Chair and Speaker presentation on non-classical nucleation pathways.

Geochemical Systems

Ionic and Microstructural Mechanisms in Next-Generation Energy Storage Materials

Rampal, Nikhil

San Francisco State University, 2025

Invited talk on mechanisms underlying next-generation energy storage.

Energy Storage

Design Principles for High-Performance Electrolytes—Overcoming Low-Temperature Challenges in Lithium-Ion Batteries

Rampal, Nikhil, Weitzner, Stephen E, Cho, Seongkoo, Orme, Christine A, Worsley, Marcus A, Wan, Liwen F

Materials Research Society, 2025

Presentation on developing battery electrolytes that function at low temperatures.

Energy Storage

Decoding the mechanistic processes that dictate battery performance using enhanced sampling simulations

Rampal, Nikhil, Adelstein, Nicole, Sun, Wenyu, Weitzner, Stephen E, Orme, Christine A, Worsley, Marcus A, Wan, Liwen F

Abstracts of Papers of the American Chemical Society, 2024

Presentation on advanced computational methods for understanding battery function.

Energy Storage

Structure and dynamics of water on Calcite (104) surface studied by quasielastic neutron scattering and molecular dynamics simulations

Rampal, Nikhil, Kroutil, Ondrej, Wang, Hsiu-Wen, Mamontov, Eugene, Biriukov, Denys, Predota, Milan, Stack, Andrew

Abstracts of Papers of the American Chemical Society, 2021

Combined experimental and computational study of water behavior at mineral surfaces.

Geochemical Systems

Amalgamation of computational and experimental studies to probe the effect of local molecular environments in aqueous salt solutions

Rampal, Nikhil, Wang, Hsiu-Wen, Biriukov, Denys, Brady, Alexander, Neuefeind, Joerg, Predota, Milan, Stack, Andrew

Pacifichem, 2021

Invited presentation on integrated approaches to understand solution chemistry.

Geochemical Systems

Chloride ion solvation, dynamics and ion-pairing interactions in concentrated aqueous solutions

Rampal, Nikhil, Wang, Hsiu-Wen, Stack, Andrew, Biriukov, Denys, Neuefeind, Joerg

Abstracts of Papers of the American Chemical Society, 257, 2019

Combined neutron diffraction and computational study of ion behavior in solution.

Geochemical Systems